首页> 外文OA文献 >Dynamical heterogeneities and defects in two-dimensional soft colloidal crystals
【2h】

Dynamical heterogeneities and defects in two-dimensional soft colloidal crystals

机译:二维软胶体晶体的动态异质性和缺陷

代理获取
本网站仅为用户提供外文OA文献查询和代理获取服务,本网站没有原文。下单后我们将采用程序或人工为您竭诚获取高质量的原文,但由于OA文献来源多样且变更频繁,仍可能出现获取不到、文献不完整或与标题不符等情况,如果获取不到我们将提供退款服务。请知悉。

摘要

In this paper we study a two-dimensional system of charged colloidal particles using Brownian dynamics simulations. We determine the phase diagram and investigate the dynamics of this system in the density regime where hexatic and solid phases are stable. We find that the dynamics in these phases is heterogeneous by means of the spontaneous formation and diffusion of highly mobile defects. We identify two key mechanisms associated with the areas of high mobility. The first mechanism involves the highly cooperative motion of a closed loop of particles which shift coherently along the loop until each particle has replaced the position of its predecessor in the chain. The second mechanism involves the spontaneous creation of vacancy-interstitial pairs which diffuse within the hexatic and solid phases. We further explore quantitatively the properties of the open-ended and closed rearrangement strings and find that in the crystal phase the string-size distribution can be approximately matched with a simple, random walk description of vacancies and interstitials on a lattice.
机译:在本文中,我们使用布朗动力学模拟研究带电胶体颗粒的二维系统。我们确定相图并研究该系统在六方相和固相稳定的密度状态下的动力学。我们发现,通过高度移动的缺陷的自发形成和扩散,这些阶段的动力学是不均匀的。我们确定了与高机动性领域相关的两个关键机制。第一种机制涉及粒子闭环的高度协作运动,该闭环沿着该环连贯地移动,直到每个粒子都替换了其前任在链中的位置。第二种机制涉及自发形成在六方相和固相中扩散的空位-间隙对。我们进一步定量研究了开放式和封闭式重排字符串的性质,发现在晶相中,字符串大小分布可以与晶格上的空位和间隙的简单随机游走近似匹配。

著录项

相似文献

  • 外文文献
  • 中文文献
  • 专利
代理获取

客服邮箱:kefu@zhangqiaokeyan.com

京公网安备:11010802029741号 ICP备案号:京ICP备15016152号-6 六维联合信息科技 (北京) 有限公司©版权所有
  • 客服微信

  • 服务号